I'm not the biggest fan of Skyward Sword but that's down to personal taste I think, so if I were you I'd do that. Definitely recommend finishing Portal 2 if you're near the end, as well as DKCR. If you had to replay just one of the games up there you have completed, (I assume the ones without brackets) I'd make it Paper Mario: The Thousand Year Door, unless you've done it to death. I meant to also vote for Super Mario Galaxy and realised too late, but I'd recommend at least one of the two Galaxy games.
I've not played Super Mario RPG and I don't remember an awful lot about the original Perfect Dark, so ignore the fact I've not voted for them.
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