Paper Mario, Super Mario RPG, Portal 2, and Super Mario Galaxy are all good games.
Before you jump into any of them though, do a quick playthrough of Star Fox 64. it's really really awesome, and really short. You'll beat it in less than a day, it's a really arcadey game, it isn't even long enough to warrant the ability to save.
Pikmin 2 isn't on the list but if you liked the first one check it out.
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